![]() ![]() In this chapter, we first highlight the critical scientific challenges as well as technological progresses for the currently studied SSEs including organic polymers, inorganic electrolytes, and the composites. However, the problems including sluggish ion transport in SSEs and the interfacial incompatibility of SSEs with electrodes significantly limit the overall performances of ASSLMBs. In addition, SSEs could in principle suppress the lithium dendrite growth and enable the utilization of lithium metal anode that is regarded as a “holy grail” of lithium batteries, in all-solid-state lithium metal batteries (ASSLMBs). ![]() Replacing flammable organic liquid electrolytes by solid-state electrolytes (SSEs) provides a fundamental solution to safety issue for lithium-ion batteries (LIBs), driven by the increasing demand of high energy density, stable cycling performance, low cost, and abuse tolerance for energy storage systems in the widespread applications of electric vehicles (EVs) and smart grids. ![]()
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